Abstract

Surface discharge plasma (SDP) combined with activated carbon (AC) was employed to eliminate dissolved organic matter from micro-polluted source water, with humic acid (HA) as the model pollutant. Synergistic effect on HA removal was observed in the SDP-AC system; HA removal efficiency reached 60.9% within 5-min treatment in the SDP-AC system with 5.0g AC addition, whereas 16.7 and 17.4% of HA were removed in sole SDP system and AC adsorption, respectively. Scanning electron microscope and Boehm titration analysis showed that chemical reactions between active species and functional groups of AC occurred. The existence of isopropanol or benzoquinone exhibited inhibitive effects on HA removal in the SDP system, while these inhibitive effects were weakened in the SDP-AC system. The influences of AC on ozone equivalent concentration and H2O2 concentration were evaluated, and there were approximately 39 and 20% decline in ozone equivalent concentration and H2O2 concentration within 6-min treatment in the SDP-AC system, respectively, compared with those in the sole SDP system. Dissolved organic carbon, specific ultraviolet absorbance, and UV absorption ratios analysis demonstrated that the SDP treatment destroyed the chromophoric groups, double bonds, and aromatic structure of HA molecules, and these destructive actions were strengthened by AC.

Full Text
Paper version not known

Talk to us

Join us for a 30 min session where you can share your feedback and ask us any queries you have

Schedule a call

Disclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.