Enhanced optoelectronic performance of 2D organic-inorganic hybrid perovskite through light-illumination.

Abstract

Improving the optoelectronic characteristics of organic-inorganic perovskites is crucial for fabrication of functional devices. Herein, we demonstrate that the optoelectronic properties of 2D organic-inorganic perovskites can be greatly improved by UV-light illumination during growth. The photoluminescence emission of the 2D perovskite exhibits a 3.1-folds increase in intensity, with a decreased trap-assisted recombination. The improved optoelectronic characteristics can be attributed to the high-quality crystallization and lattice expansion induced by the UV-light illumination. Moreover, the optimized 2D perovskites enable the fabrication of photoconductive devices with improved optoelectronic responses. This work indicates that light illumination is a novel and convenient approach for engineering the fabrication of 2D organic-inorganic hybrid perovskites, which advocates great promise for achieving high-performance functional devices.