Enhanced magnetic anisotropy induced by praseodymium ferromagnetic order and anomalous transport properties in PrMn2Ge2 single crystals

Abstract

Anisotropic magnetization and anomalous electrical transport properties of flux-grown $\mathrm{Pr}{\mathrm{Mn}}_{2}{\mathrm{Ge}}_{2}$ single crystals were investigated. The grown crystals exhibit strong magnetic anisotropy with easy magnetization along the $c$ axis. Linear magnetoresistance (MR) and a conventional anomalous Hall effect (AHE) are observed for $H\text{//}c$ and $I\text{//}b$ in contrast to a nonlinear positive MR and a large planar topological Hall effect (PTHE) observed for $H\text{//}a$ and $I\text{//}b$. The anisotropy of the magnetic and electrical transport properties is increased as temperature decreases because magnetic ordering of Pr atoms brings about an increase of the saturation magnetic field of nonlinear MR and the critical field for the maximum values of PTHE. A scaling analysis using the Tian-Ye-Jin model suggests that the AHE in this compound has a larger intrinsic contribution compared to the extrinsic contribution. The nonlinear positive MRs are attributed to the field-induced nontrivial spin textures. The PTHE is related to the real-space skyrmionic bubbles and the noncoplanar spin texture with nonzero spin chirality. These results demonstrate a magnetic field induced anisotropic magnetoresistance and Hall resistivity and its tunability by the ferromagnetic ordering of rare earth atoms in conical-ordered magnets.