Abstract

The transformation of a moderately excited heavy nucleus into two excited fission fragments is modeled as a strongly damped evolution of the nuclear shape. The resulting Brownian motion in the multi-dimensional deformation space is guided by the shape-dependent level density which has been calculated microscopically for each of nearly ten million shapes (given in the three-quadratic-surfaces parametrization) by using a previously developed combinatorial method that employs the same single-particle levels as those used for the calculation of the pairing and shell contributions to the five-dimensional macroscopic-microscopic potential-energy surface. The stochastic shape evolution is followed until a small critical neck radius is reached, at which point the mass, charge, and shape of the two proto-fragments are extracted. The available excitation energy is divided statistically on the basis of the microscopic level densities associated with the two distorted fragments. Specific fragment structure features may cause the distribution of the energy disvision to deviate significantly from expectations based on a Fermi-gas level density. After their formation at scission, the initially distorted fragments are being accelerated by their mutual Coulomb repulsion as their shapes relax to their equilibrium forms. The associated distortion energy is converted to additional excitation energy in the fully accelerated fragments. These subsequently undergo sequential neutron evaporation which is calculated using again the appropriate microscopic level densities. The resulting dependence of the mean neutron multiplicity on the fragment mass, as well as the dependence of on the initial excitation energy of the fissioning compound nucleus, exhibit features that are similar to the experimentally observed behavior, suggesting that the microscopic energy sharing mechanism plays an important role in low-energy fission.

Highlights

  • Microscopic shape-dependent level densityIn Ref. [1] a method was developed for microscopic calculations of level densities for deformed nuclei and it has been adapted to the fission process [2]

  • We illustrate here how shape-dependent microscopic level densities may be used to refine the theoret- ical modeling of nuclear fission

  • The use of microscopic level densities is well- suited for describing the dependence of the shape evolution on the total excitation energy of the fissioning system because the microscopic pairing and shell e↵ects automatically subside as the energy is raised, without the need for any adjustable parameters

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Summary

Microscopic shape-dependent level density

In Ref. [1] a method was developed for microscopic calculations of level densities for deformed nuclei and it has been adapted to the fission process [2]. For a specified shape χ, the single-particle levels for protons and neutrons needed for the combinatorial calculation of the level density are obtained by solving the Schrödinger equation in the associated foldedYukawa potential. These are the same levels as those previously used in Ref. For each many-particle-many-hole excitation, a BCS pairing calculculation is carried out for neutrons and protons separately, yielding the associated correlated energy intrinsic state, n (χ). For each shape χ, the resulting states are binned according to their energy Ei and their total angular momentum I; the bin width was taken as ∆E = 200 keV. The sensitivity of the results to the bin width has been tested and it was found that a doubling or tripling of ∆E has no discernable e↵ect on the calculated observables

Brownian shape evolution
Scission
Conclusion
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