Abstract
Abstract Naphthalene-TCNB charge transfer crystals doped with 2-methyl naphthalene illuminated by visible light give rise to triplet traps which have been identified by EPR and ENDOR spectroscopy as 2-methyl naphthalene-TCNB CT complexes in their first excited triplet state. The complete hyperfine tensors of all the 2-methyl naphthalene protons have been obtained by analysis of the variation of the ENDOR frequencies with the crystal orientation in the magnetic field. The structure of the CT complex, the spin distribution and the CT character are discussed.
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