Enantiospecific state transfer for gaseous symmetric-top chiral molecules

Abstract

We study the enantio-specific state transfer in a four-level model for symmetric-top chiral molecules. Such a model is formed by coupling the electric-dipole transitions among four appropriate working states with three electromagnetic fields. It includes two cyclic three-level substructures, where the overall phases differ by $\pi$ with enantiomers and reflect the chirality dependence of the molecule. Based on this four-level model, two dynamic ways are proposed to achieve the approximately perfect enantio-specific state transfer for symmetric-top chiral molecules.