Abstract
An efficient enantioselective total synthesis of pyrrolo-[2,1-c][1,4]benzodiazepine (PBD) monomers (S)-(−)-barmumycin and (S)-(+)-boseongazepine B was achieved through a stereocontrolled strategy, which relies on a proline catalysed asymmetric α-amination and ester α-ethylenation.
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