Abstract

X-band electron magnetic resonance (EMR) spectra were recorded at the temperature range of 115⩽ T⩽600 K on powdered samples of single crystalline La 0.9Ca 0.1MnO 3 and polycrystalline La 0.1Ca 0.9MnO 3 manganites, having a mixed magnetic structure in the ground state, which comprises canted antiferromagnetic matrix and nanometer-scale ferromagnetic clusters. A model of the magneto-impurity states for excess holes and electrons, which emerge in the considered compounds due to A-site cation substitution, was used for modeling their paramagnetic susceptibility and spin dynamics measured by means of EMR.

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