Abstract
Electric field control can actively, dynamically, and repeatably influence the interface friction behavior. The unique properties of two-dimensional (2D) ZIF-8 make it a promising lubricating material for electromechanical devices. The study on the electrotunable superlubricity of 2D ZIF-8 is carried out under longitudinal and transverse electric fields respectively, resulting in an order of magnitude variation in friction coefficient (μ: 0.0037–0.0124). Through the experiments and simulation, the regulation mechanism of electric fields on the lubricating properties of 2D ZIF-8 is attributed to the coupling effect of adhesion regulation and out-of-plane deformation regulation: The weakening of anchoring effect reduces the adhesion between probe and 2D ZIF-8; the tight binding of interfacial charge under longitudinal electric field as well as the increase in surface stiffness caused by lattice tension under transverse electric field, both restrain the out-of-plane deformation during friction. The electrotunable superlubricity of 2D ZIF-8 helps achieve rapid and flexible adjustment of the friction interface in electro-mechanical systems under charged conditions, illuminating the future development prospects for intelligent control.
Published Version
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