Abstract
Between 330 and 400 nm the 2+1 REMPI spectrum of SiCl 3 exhibits two overlapping vibrational progressions composed of >30 members and one vibrational progression composed of five members. These band systems, labeled F, G, and H, are tentatively assigned to three distinct Rydberg states that reside between 50100 and 59 600 cm -1 . The vibrational progressions have an average spacing of ω 2 =262 cm -1 and are assigned to the ν 2 umbrella modes of the Rydberg states
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