Electronic level structure of Th+ in the range of the Th229m isomer energy

Abstract

Using resonant two-step laser excitation of trapped $^{232}\mathrm{Th}^+$ ions, we observe 166 previously unknown energy levels of even parity within the energy range from 7.8 to 9.8 eV and angular momenta from $J=1/2$ to $7/2$. We also classify the high-lying levels observed in our earlier experiments by the total angular momentum and perform ab-initio calculations to compare their results with the observed level density. The observed levels can be relevant for the excitation or decay of the $^{229m}\mathrm{Th}$ isomeric nuclear state which lies in this energy range. The high density of electronic levels promises a strongly enhanced electronic bridge excitation of the isomer in $^{229}\mathrm{Th}^+$.