Abstract
The dynamics of a cold photoexcited electron–hole system created by resonant excitation with picosecond optical pulses are studied by time-resolved emission and pump–probe measurements. A rapid build-up of strong metallic reflection in the mid-infrared region was observed, which indicates the creation of electron–hole plasma via the exciton or biexciton Mott transition. Transient reflection spectra clearly show the transformation of high-density electron–hole plasma into a metallic colloid-like state within 10 ps. In the meantime, broad plasma emission turns to a narrow emission band, in which the spectral profile does not change within several tens of picoseconds. These features in the emission spectra disappear when switched to the band-to-band excitation. An analysis of the reflection and emission spectra reveals that the density of metastable electron–hole liquid is as high as 10 20 cm −3. This indicates that the plasma formation via the Mott transition is crucial to eliminate excess heating for reaching the low-temperature states of an electron–hole ensemble.
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a callDisclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.
