Abstract
The electron spin resonance spectra of several previously unobserved alkyl- and cycloalkyl-aromatic radical cations were obtained in a flow system, and the ratio of the methylene hyperfine splittings to the corresponding methyl hydrogen splittings was measured. These ratios, which ranged from 0.46 to 1.79, were rationalized on the basis of the preferred geometrical conformations of these molecules.
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