Abstract
The EPR results of the selectively deuteriated solute cations 2-methylbutane, 3-methylpentane and 3-methylhexane (2MB+, 3MP+ and 3MHX+) produced in halocarbon matrices (perfluoro-2-methylpentane, CFCl3, CF2ClCFCl2, CF2BrCF2Br and CF2BrCFBrCl) have been studied by means of INDO-MO calculations. The structures of the cations were found to depend on the matrix. The INDO method has shown that the structural changes can be reasonably interpreted on the basis of the structures of 2MB+.
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