Abstract
Hyperfine splitting parameters have been measured for the neutron-deficient odd-mass polonium isotopes and isomers 193?203Pog,m, 209,211Po. The measurement was performed at the ISOLDE (CERN) online mass separator using the in-source resonance ionization spectroscopy technique. The magnetic dipole moments ? and spectroscopic electric quadrupole moments QS have been deduced. Their implication for the understanding of nuclear structure in the vicinity of the closed proton shell at Z = 82 and the neutron mid-shell at N = 104 is discussed. For the most neutron-deficient nuclei (A = 193,195,197), a deviation of ? and QS from the nearly constant values for heavier polonium nuclei was observed. Particle-plus-rotor calculations with static oblate deformation describe the electromagnetic moments for these nuclei well, provided a gradual increase of a mean deformation when going to lighter masses is assumed for the polonium nuclei with A < 198.
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