Abstract
The electrochemical behaviour of the new Nb IV derivatives [Nb(η 5-C 5H 5) 2(LL)][PF 6] 2 where LL = 2,2′-bipy The structure of the new [Nb(η 5-C 5H 5) 2(bpy)][PF 6] 2 ( 1) and of the known related compounds [Mo(η 5-C 5H 5) 2 An extended-Hückel molecular-orbital study of the bonding of these complexes showed the absence of back donation to the low-energy, empty orbitals of
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