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Abstract
Introduction of bis(fluorosulfonyl)imide (FSI) as an anion to an ambient-temperature ionic liquid electrolyte based on 1-ethyl-3-methylimidazolium and lithium (Li) as cations can provide a reversible Li intercalation into a graphitized electrode, while the intercalation is completely irreversible without FSI. Laser desorption/ionization mass spectroscopy and ac impedance spectroscopy suggest that FSI-coordinated Li+ is facilely mobile even without any solvents and is reversibly accessible to a graphite interior.
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