Electrical characterization of positive and negative pulsed nanosecond discharges in water coupled with time-resolved light detection

Abstract

Electrical discharge in liquids is a research field that has great potential in environmental and technological applications. Depending on the experimental conditions (liquid nature, interelectrodes distance, applied voltage, pulse width, etc.), various discharge modes can be obtained. The involved physical processes have relatively fast spatiotemporal dynamics and, therefore, are not well understood. In this study, we report the electrical characterization, coupled with time-resolved light detection (using a photomultiplier, PM, tube), of positive and negative pulsed nanosecond spark discharges in de-ionized water using copper electrodes (distanced by ∼50 μm) in a pin-to-plate configuration. A detailed analysis of the current–voltage waveforms during the pre-breakdown and the breakdown phases is shown, and we found that the pre-breakdown phase depends on the high voltage magnitude only for positive polarity. On the other hand, the PM signals showed dependence on the voltage magnitude and on the pulse width, and various emission phases are observed. These phases can be related to the discharge power and/or to the discharge current. Filtered PM signals at various wavelengths are also acquired, and their temporal dynamics are discussed regarding the discharge conditions.