Abstract

In this paper, we present an original model to describe the role of the elastic interactions in cooperative spin crossover compounds that switch between the low-spin (diamagnetic) to high-spin (paramagnetic) states. The interactions are analyzed by the way of their effect on thermal hysteresis loop at different external pressures and on the first-order reversal curves distribution. A comparison with experimental data for the pure spin crossover compound [Fe(btr) <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">2</sub> (NCS) <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">2</sub> ]H <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">2</sub> O is provided.

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