Abstract
Generation of entangled photons in nonlinear media constitutes a basic building block of modern photonic quantum technology. Current optical materials are severely limited in their ability to produce three or more entangled photons in a single event due to weak nonlinearities and challenges achieving phase-matching. We use integrated nanophotonics to enhance nonlinear interactions and develop protocols to design multimode waveguides that enable sustained phase-matching for third-order spontaneous parametric down-conversion (TOSPDC). We predict a generation efficiency of 0.13 triplets/s/mW of pump power in TiO2-based integrated waveguides, an order of magnitude higher than previous theoretical and experimental demonstrations. We experimentally verify our device design methods in TiO2 waveguides using third-harmonic generation (THG), the reverse process of TOSPDC that is subject to the same phase-matching constraints. We finally discuss the effect of finite detector bandwidth and photon losses on the energy-time coherence properties of the expected TOSPDC source.
Highlights
Optical quantum technologies [1] often rely on nonlinear optical crystals pumped with coherent radiation to generate light with non-classical properties, including entanglement
We experimentally verify our device design methods in TiO2 waveguides using third-harmonic generation (THG), the reverse process of thirdorder spontaneous parametric down-conversion (TOSPDC) that is subject to the same phase-matching constraints
Entangled states of light containing three or more photons are currently built interferometrically starting from entangled photon pairs or single photons [2], with entangled pairs typically generated via spontaneous parametric down-conversion (SPDC) [8], biexciton decay [9], and spontaneous four-wave mixing [10]
Summary
Optical quantum technologies [1] often rely on nonlinear optical crystals pumped with coherent radiation to generate light with non-classical properties, including entanglement. The production of entangled photon triplets via cascaded SPDC has been demonstrated [13,14,15], with generation efficiencies on the order of 10−2 triplets/s/mW pump power [14]. Third-order spontaneous parametric down conversion (TOSPDC), when one pump photon splits into three signal photons, can generate entangled photon triplets. Sustained phasematching for widely-spaced wavelengths can be achieved using strong dispersion in nonfundamental waveguide modes. These remarkable improvements over bulk materials indicate that integrated nanophotonic waveguides can enable efficient TOSPDC. We propose a protocol to optimize efficient generation of entangled photon triplets via TOSPDC in nanophotonic waveguides. We calculate the temporal coherence properties of TOSPDC sources in coincidence measurements, taking into account finite detector bandwidths and propagation losses
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