Abstract

Experimental research on non-critical phase-matching fourth harmonic generation with ADP and DKDP crystals are reported. The characteristics of 2ω-to-4ω efficiency as function of incident angle, crystal temperature and input 2ω intensity have been investigated in detail, and the 2ω-to-4ω conversion efficiency has been demonstrated up to 84.1% with ADP crystal and 85.1% with DKDP crystal, respectively. Nevertheless, the spatial non-uniformity of rapid grown DKDP crystal has to be improved while the temperature control uniformity should be upgraded for ADP crystal to realize large aperture high efficiency fourth harmonic generation.

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