Abstract

The neutron-rich $^{122-131}$Sb isotopes were produced as fission fragments in the reaction $^{9}$Be($^{238}$U,~f) with 6.2 MeV/u beam energy. An unique setup, consisting of AGATA, VAMOS++ and EXOGAM detectors, was used which enabled the prompt-delayed gamma-ray ($\gamma$) spectroscopy of fission fragments in the time range of 100 ns - 200 $\mu$s. New isomers, prompt and delayed transitions were established in the even-A $^{122-130}$Sb isotopes. In the odd-A $^{123-131}$Sb isotopes, new prompt and delayed $\gamma$-ray transitions were identified, in addition to the confirmation of the previously known isomers. The half-lives of the isomeric states and the $B(E2)$ transition probabilities of the observed transitions depopulating these isomers were extracted. The experimental data was compared with the theoretical results obtained in the framework of Large-Scale Shell-Model (LSSM) calculations in a restricted model space. Modifications of several components of the shell model interaction were introduced to obtain a consistent agreement with the excitation energies and the $B(E2)$ transition probabilities in neutron-rich Sn and Sb isotopes. The isomeric configurations in Sn and Sb were found to be relatively pure. Further, the calculations revealed that the presence of a single valence proton, mainly in the $g_{7/2}$ orbital in Sb isotopes, leads to significant mixing (due to the $\nu\pi$ interaction) of: (i) the neutron seniorities ($\upsilon_{\nu}$) and (ii) the neutron angular momentum ($I_{\nu}$). The above features have a weak impact on the excitation energies, but have an important impact on the $B(E2)$ transition probabilities. In addition, a constancy of the relative excitation energies irrespective of neutron seniority and neutron number in Sn and Sb was observed.

Highlights

  • The Sn isotopes, with basically a spherical shape, span between two doubly magic nuclei, the neutron-deficient 100Sn (Z = N = 50) and the neutron-rich 132Sn (Z = 50, N = 82).A constant trend, as a function of neutron number, in the excitation energies (EX ) of the 2+ state and the parabolic shape of the reduced electricquadrupole transition probabilities [B(E 2; 2+ → 0+)], was observed for the even-A Sn isotopes [1,2]

  • The neutron-rich 122–131Sb isotopes were produced as fission fragments in the reaction 9Be(238U, f ) with 6.2 MeV/u beam energy

  • The neutron-rich 122–131Sb isotopes were produced as fission fragments in the reaction 9Be (238U, f ) with 6.2 MeV/u beam energy

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Summary

Introduction

A constant trend, as a function of neutron number, in the excitation energies (EX ) of the 2+ state and the parabolic shape (with a dip around N = 66) of the reduced electricquadrupole transition probabilities [B(E 2; 2+ → 0+)], was observed for the even-A Sn isotopes [1,2]. Purpose: Benchmark the reproducibility of the experimental observables, like the excitation energies (EX ) and the reduced electric-quadrupole transition probabilities [B(E 2)], with the results obtained from shell-model interactions for neutron-rich Sn and Sb isotopes with N < 82. Modifications of several components of the shell-model interaction were introduced to obtain a consistent agreement with the excitation energies and the B(E 2) transition probabilities in neutron-rich Sn and Sb isotopes. A constancy of the relative excitation energies irrespective of neutron seniority and neutron number in Sn and Sb was observed

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Discussion
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