Abstract

The effects of isotropic artifical defects, introduced via fast neutron (E > 0.1 MeV) irradiation, on the physical properties of differently (Co, P and K) doped BaFe2As2 superconducting single crystals were studied. The Co- and P-doped single crystals showed a second peak in the magnetization curve (fishtail effect) in the pristine state. Significant variations in the radiation-induced changes in the critical current density Jc were observed in the different types of crystal, while the irreversibility fields did not change remarkably. The highest Jcs were obtained for the K-doped crystal, exceeding 3 × 1010 Am−2 (T = 5 K, B = 4 T) and remaining above 8.5 × 109 Am−2 at 30 K and 1 T. The pinning force was analyzed to compare the pinning mechanisms of the individual samples. While distinct differences were found before the irradiation, the same pinning behavior prevails afterwards. The pinning efficiency η = Jc/Jd was estimated from the depairing current density Jd. η was similar in all irradiated crystals and comparable to the value in neutron irradiated cuprates, suggesting that the huge critical current densities measured in the irradiated K-doped crystal are due to its large depairing current density, making this compound the most promising for applications.

Highlights

  • Tc was evaluated from the onset of the diamagnetic response arising from superconductivity (Tconset)

  • The transition temperatures of all pristine crystals were close to the highest values reported for the respective bulk systems

  • The difference Tconset,pris − Tconset,irr = δT c is used to illustrate the effect of fast neutron irradiation on the transition temperature of the differently doped single crystals

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Summary

Introduction

The values obtained in this study agree with previous results on the effects of fast neutron irradiation on Tc of Co-doped single crystals[25] and other iron-based compounds[14]. The Co-doped crystal has the highest critical current densities in the pristine state, while the K-doped crystal shows the lowest Jcs prior to fast neutron irradiation.

Results
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