Abstract
The effects of inorganic substances on water splitting in ion-exchange membranes (IEMs) were investigated. In this study, iron hydroxide/ oxide and silica sol were immobilized on the surface of the IEMs. The water-splitting capabilities of the metal-embedded cation-exchange membranes were 10 4–10 5 times greater than those of the virgin membranes at the same current density. Similarly, silica sol (i.e., SiOH groups) deposited on the anion-exchange membrane surface also drastically increased the proton transport numbers. It was thought that the bipolar structure consisting of H- and OH-affinity groups immobilized on the IEM surface increased water-splitting due to the enhancement of water polarization with the help of strong electric fields. This study revealed that metal oxides or silica groups (SiOH), as well as metal hydroxides, can be used as catalysts for water splitting.
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