Abstract

Higher-order multiscale structures are proposed to predict the effective elastic properties of 3-phase particle reinforced composites by considering the probabilistic spherical particles spatial distribution, the particle interactions, and utilizing homogenization with ensemble volume average approach. The matrix material, spherical particles with radius a<sub>1</sub>, and spherical particles with radius a<sub>2</sub>, are denoted as the 0<sup>th</sup> phase, the 1<sup>st</sup> phase, and the 2<sup>nd</sup> phase, respectively. Particularly, the two inhomogeneity phases are different particle sizes and the same elastic material properties. Improved higher-order (in ratio of spherical particle sizes to the distance between the centers of spherical particles) bounds on effective elastic properties of 3-phase particle reinforced proposed Formulation II and Formulation I derive composites. As a special case, i.e., particle size of the 1<sup>st</sup> phase is the same as that of the 2<sup>nd</sup> phase, the proposed formulations reduce to 2-phase formulas. Our theoretical predictions demonstrate excellent agreement with selected experimental data. In addition, several numerical examples are presented to demonstrate the competence of the proposed frameworks.

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