Abstract
Potassium dihydrogen phosphate (KDP) single crystal was doped with disodium tetraborate decahydrate (or borax), L-alanine, and disodium ethylenediaminetetraacetate (or disodium EDTA) with 0.05 mol%, 9 mol%, and 2 mol% concentration in the aqueous solution, respectively. These crystals were fabricated by the temperature reduction method incorporating the Sankaranarayanan-Ramasamy technique and were grown onto seed crystals that were inclined at the type I phase-matching angle to the vertical. Each doped KDP single crystal rod was cut into three parts: the bottom, the middle, and the top, which were related to the fabrication temperature range of 50–40 °C, 40–30 °C, and 30–20 °C, respectively. The effect of the additives on the growth and optical properties of KDP crystals was evaluated through Ultraviolet–Visible spectroscopy, Raman spectroscopy, X-Ray Diffraction analysis, Energy-Dispersive X-ray spectroscopy, and Second Harmonic Generation measurement. The hydroxyl impurities have improved the optical properties of KDP crystals by contributing more hydrogen bonds to the KDP lattice. The doped KDP crystals increased SHG efficiency by 1.19 to 2.36 times compared with pure KDP crystals.
Published Version
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