Abstract

RbGd2Fe4As4O2 is a newly discovered self-hole-doped stoichiometric superconductor, which has a hybrid structure with separated double FeAs layers and exhibits a high superconducting transition temperature Tc = 35 K. Here, we report the effect of pressure (P) on its Tc and normal-state transport properties by measuring the temperature dependence of resistivity ρ(T) under various pressures up to 14 GPa with a cubic anvil cell apparatus. We found that the Tc is suppressed monotonically to ca. 12.5 K upon increasing pressure to 14 GPa with a slope change of Tc(P) at around 4 GPa. In addition, the low-temperature normal-state ρ(T), which is proportional to Tn, also evolves gradually from a non-Fermi-liquid with n = 1 at ambient pressure to a Fermi liquid with n = 2 at P ⩾ 4 GPa. Accompanying with the non-Fermi-liquid to Fermi-liquid crossover, the quadratic temperature coefficient of resistivity, which reflects the effective mass of charge carriers, also experiences a significant reduction as commonly observed in the vicinity of a magnetic quantum critical point (QCP). Our results indicate that the stoichiometric RbGd2Fe4As4O2 at ambient pressure might be located near a QCP such that the enhanced critical spin fluctuations lead to high-Tc superconductivity. The application of pressure should broaden the electronic bandwidth and weaken the spin fluctuations, and then restore a Fermi-liquid ground state with lower Tc.

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