Abstract
Oxygen-rich combustion is a new type of clean combustion technology with important application prospects. In this work, the effects of oxygen-rich combustion on soot formation in the propane/(O2+N2) laminar flow coaxial jets diffusion flame were numerically investigated by using the detailed gas-phase chemical reaction model with the mechanism of tetracyclic aromatic hydrocarbons and the complex thermodynamic properties and transport characteristics parameters. Soot surface growth follows the hydrogen-abstraction-carbon-addition (HACA) model. A hybrid gas-phase mechanism was adopted, which contains a DLR-based polycyclic aromatic hydrocarbons (PAHs) formation, growth model and a gas-phase model. Results show that the oxygen-rich combustion has a great influence on the flame temperature, especially the high temperature region. With the increase of oxygen concentration, the soot formation region of flame broadens and the maximum of soot volume fraction increase from 3.95 ppm to 10.87 ppm. The extra oxygen makes PAHs increased around the nozzle, leading to larger rate in early soot nucleation and surface growth, eventually more soot yield.
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