Effect of Lorentz local field correction on propagation of ultrashort laser pulse in one-dimensional para-nitroaniline (PNA) molecules

Abstract

This paper investigates the effect of Lorentz local field correction (LFC) on the propagation of ultrashort laser pulses in a para—nitroaniline molecular medium under resonant and nonresonant conditions by solving numerically the full-wave Maxwell—Bloch equations beyond slowly-varying envelope approximation and rotating-wave approximation. The effect of the LFC is considerably obvious when pulses with large areas propagate in the dense molecular medium. In the case of resonance, the group velocity of the sub-pulses split from the incident pulse along propagation is severely decreased by the LFC, especially for the latest sub-pulse. However, in the case of nonresonance, the influence of the LFC on the temporal evolution of the pulse is less obvious and lacks homogeneity with an increase in incident pulse area, propagation distance and molecular density.