Abstract

The AlOx-based resistive switching memory device is fabricated by an oxidation diffusion process that involves depositing an Al film on an ITO substrate and annealing at 400 °C in a vacuum. An AlOx interface layer with a thickness of ~ 20 nm is formed as a resistance switching layer. Bipolar and unipolar resistive switching (RS) behaviours are obtained when the compliance current is limited (≥ 1 mA). In the unipolar RS behaviour, the devices fail to perform set/reset cycles at a low temperature (40 K), which suggests that Joule heating is essential for the unipolar RS behaviour. In the bipolar RS behaviour, the abrupt reset transforms into a gradual reset with decreasing temperature, which suggests that Joule heating affects the rupture of the conductive filament. In addition, the conductive mechanisms in the high-resistance state and low-resistance state are revealed by the temperature dependence of the I-V curves. For the low-resistance state, the conduction mechanism is due to the electron hopping mechanism, with a hopping activation energy of 9.93 meV. For the high-resistance state, transport mechanism is dominated by the space-charge-limited conduction (SCLC) mechanism.

Highlights

  • Resistive switching random access memory (RRAM) has attracted extensive attention as one of the most promising candidates for next-generation non-volatile memory [1–4]

  • We investigate the conductive mechanism by the temperature dependence of the current for high-resistance state (HRS) and lowresistance state (LRS)

  • To check the microstructure changes after annealing the Pt/Al/ITO devices, high-resolution transmission electron microscopy (HRTEM) is used to check the region between the Al and ITO glass substrates

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Summary

Introduction

Resistive switching random access memory (RRAM) has attracted extensive attention as one of the most promising candidates for next-generation non-volatile memory [1–4]. Zhang et al Nanoscale Research Letters (2020) 15:11 currents, Joule heating is used to explain the rupture conductive filaments in the reset process of the unipolar RS behaviour. The use of Joule heating to assist in rupturing conductive filaments in the reset process is proposed for the bipolar RS behaviour. The effect of Joule heating is well verified by placing the device at different temperatures. The performance effect at different temperatures for AlOx RRAM is investigated. A deeper understanding of the effect of Joule heating in the resistive switching process is important and necessary. We investigate the conductive mechanism by the temperature dependence of the current for high-resistance state (HRS) and lowresistance state (LRS)

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