Abstract
The effect of imprisonment of radiation in sodium vapor on the measured lifetime of the $3 ^{2}P$ states has been investigated in an experiment in which the atoms in the vapor were excited with 10-nsec pulses of resonance radiation and the elapsed times between the exciting and the fluorescent pulses were recorded using a time-to-amplitude converter and kicksorter. At vapor densities below ${10}^{10}$ atoms/${\mathrm{cm}}^{3}$, where there is no multiple scattering, the measured lifetime reaches a constant value of (1.63\ifmmode\pm\else\textpm\fi{}0.04)\ifmmode\times\else\texttimes\fi{}${10}^{\ensuremath{-}8}$ sec, equal to the natural lifetime of the $3 ^{2}P$ states. In the density range ${10}^{9}$-${10}^{13}$ atoms/${\mathrm{cm}}^{3}$, the variation of the effective lifetime with the vapor density is in good agreement with the predictions of Milne's theory of radiation trapping; agreement with Holstein's theory is observed only in the range ${10}^{12}$-${10}^{13}$ atoms/${\mathrm{cm}}^{3}$. The results of a subsidiary Hanle experiment show that a multiply scattered photon of sodium resonance fluorescence loses its original polarization and that, at high sodium vapor pressure, coherence is not preserved.
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