Abstract
Solid catalytic materials play a key role in the development of industrial chemistry, showing important advantages over liquid materials thanks to their easier separation from the reaction liquid medium, their reusability and stability, and their environmentally friendly character [...]
Highlights
Solid catalytic materials play a key role in the development of industrial chemistry, showing important advantages over liquid materials thanks to their easier separation from the reaction liquid medium, their reusability and stability, and their environmentally friendly character
Transient measurement techniques have been applied for the kinetic investigation of the reaction mechanism, using diffuse reflectance infrared spectroscopy (DRIFT) and mass spectrometry
Main aspects of reaction mechanisms based on copper exposure, the copper–zirconia interphase, the zirconia surface hydroxylation degree and acid base properties are discussed, considering their impact on the surface hydrogen and intermediates mobility and on the electronics and stability of the copper phase
Summary
Solid catalytic materials play a key role in the development of industrial chemistry, showing important advantages over liquid materials thanks to their easier separation from the reaction liquid medium, their reusability and stability, and their environmentally friendly character. In situ and operando characterization techniques represent a suitable tool to identify and quantify the nature and functionality of surface adsorption active sites and, for correlating the catalytic behaviour with the surface properties of the investigated systems [1].
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