Abstract
Coherent effects produced by high-intensity pumping on aR (6, 0) in NH 3 are investigated for both the pure gas and for mixtures with an inert buffer gas. Two different Raman transitions are observed. One is the usual directly pumped Raman transition, and the other is pumped indirectly since it first requires a large population transfer to the upper vibrational level. This population transfer also creates inversion gain, shifted away from line center due to ac Stark shifts, on both transitions. Raman gain coefficients of 10 percent ċ cm-1and inversion gain coefficients > 2 percent ċ cm-1are observed, and compared to a combined density-matrix and rate-equation model.
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a callDisclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.
