Abstract
Abstract The dissociative excitation of HCN and DCN producing CN(B2Σ+) in collision with Ar(3P0,2) was investigated in a flowing afterglow. The Δν = 0, −1, and −2 sequences of the CN(BX) violet emission were analyzed by computer simulation, and the vibrational and rotational distributions of the CN(B2Σ+) fragment were obtained. Possible reaction pathways were studied on the basis of a linear surprisal analysis of the observed distributions and their isotope effects.
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