Abstract

Dynamic surface wetting of particles in contact with droplet is a complex phenomenon ubiquitously encountered in many multiphase systems of industrial importance. In this study, we address this aspect by investigating impact behavior of a water droplet (diameter = 2.9 ± 0.1 mm) in the Weber number (We) range from ~4 to 104 on a stationary spherical brass particle (diameter = 10 mm) with and without heat transfer using a combination of high speed imaging and computational fluid dynamics (CFD) modeling approach. In cold state interactions (20°C), droplet exhibited oscillatory interfacial motion comprising periodic spreading and recoiling motion. Interactions involving heat transfer were studied in film boiling regime (350°C) and two outcomes were noted—droplet rebound and disintegration. A coupled Level Set and Volume of Fluid (VOF) approach based multiphase CFD model was utilized to predict the dynamic spread ratio and transient evolution of droplet shape during the interaction. To capture the complex contact line motion realistically, a continuous time varying profile of experimentally measured dynamic contact angles was used as a wall boundary condition for the cold interactions which provided good agreement with experimentally measured droplet spread ratio. In film boiling regime, droplet spread ratio was correlated to impact Weber number and a power law trend was obtained. Rebound and disintegration outcomes were characterized by the droplet-particle contact time. For simulating interactions in film boiling regime, a constant contact angle in the limit of super-hydrophobic surface was implemented in the CFD model to account for the apparent non-wetting effect due to vapor film formation at the contact area. A sensitivity analysis was performed involving three different contact angle boundary conditions (θs = 150, 160, and 170°) to represent the surface hydrophobicity. CFD model predicted interaction outcomes and droplet spread ratios were in reasonable agreement with the experiment at different impact Weber numbers. Increase in spherical surface heat flux and corresponding rise in droplet temperature at different impact Weber numbers were also quantified which showed an increasing trend up to a critical Weber number for droplet disintegration.

Highlights

  • Dynamic wetting of particle surface is an important research aspect in the area of multiphase flows

  • After reaching the maximum spreading state, all three cases exhibit recoiling phase indicated by a sharp decline in the spread ratio parameter which is more prominent in the higher Weber number cases (We ∼ 12 and 19)

  • This could be explained by the greater rate of conversion of surface energy into kinetic energy in the recoiling phase due to more interfacial area produced at higher Weber number

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Summary

Introduction

Dynamic wetting of particle surface is an important research aspect in the area of multiphase flows. Ample process applications such as spray coating of tablets in pharmaceutical applications (Hardalupas et al, 1999), vaporization of vacuum gas oil feed droplets in contact with catalyst particles in fluid catalytic cracking unit (Ge and Fan, 2007; Mitra et al., 2013, 2015, 2016, 2017; Nguyen et al, 2015; Banitabaei and Amirfazli, 2017), spray drying (Charalampous and Hardalupas, 2017), thermal cracking of bitumen feed in fluid coking unit, scrubbing of particulate matters from off-gas stream (Mitra et al., 2013, 2015, 2016, 2017) require adequate surface wetting of particles. The spread-out lamella is retracted by the restoring surface tension force to minimize the surface area and initiates the recoiling phase

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