Abstract

Measurements of cloud droplet spectra performed with the Fast-Forward Scattering Spectrometer Probe during the Small Cumulus Microphysics Study (1995) are analyzed. Fifty cloud samples with narrow droplet spectra are selected. They are characterized by values of liquid water content slightly below the adiabatic value. Each observed spectrum is then compared to a narrow adiabatic spectrum predicted at the same level with the current theory of condensational growth in an adiabatic cloud cell, initialized with a reference spectrum measured right above the activation level, at cloud base. Broadening is characterized for each observed spectrum by the probability density function of condensational growth expressed as the Lagrangian integral of the ratio of supersaturation to vertical velocity, along the droplet trajectories. In particular it appears that the derived density functions show high probabilities of very low and very large values of condensational growth. The large values are related to a high relative density of big droplets in the measured spectra, higher than predicted by the adiabatic model. The contribution of the instrument to this feature is examined with a model of probe functioning. The simulations suggest that most of those big droplets are instrumental artifacts. The remaining broadening is parameterized by a linear relationship between the mean value and the standard deviation of the density function of condensational growth. This result will be used to examine the respective contributions to spectra broadening of microscale heterogeneities of the droplet concentration, in Part II, and of the mixing processes, in Part III of this series.

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