Abstract
Abstract. Aerosol–cloud interactions are complex, including albedo and lifetime effects that cause modifications to cloud characteristics. With most cloud–aerosol interactions focused on the previously stated phenomena, there have been no in situ studies that focus explicitly on how aerosols can affect large-scale (centimeters to tens of meters) droplet inhomogeneities within clouds. This research therefore aims to gain a better understanding of how droplet inhomogeneities within cumulus clouds can be influenced by in-cloud droplet location (cloud edge vs. center) and the surrounding environmental aerosol number concentration. The pair-correlation function (PCF) is used to identify the magnitude of droplet inhomogeneity from data collected on board the Center for Interdisciplinary Remotely Piloted Aircraft Studies (CIRPAS) Twin Otter aircraft, flown during the 2006 Gulf of Mexico Atmospheric Composition and Climate Study (GoMACCS). Time stamps (at 10−4 m spatial resolution) of cloud droplet arrival times were measured by the Artium Flight phase-Doppler interferometer (PDI). Using four complete days of data with 81 non-precipitating cloud penetrations organized into two flights of low-pollution (L1, L2) and high-pollution (H1, H2) data shows enhanced inhomogeneities near cloud edge as compared to cloud center for all four cases. Low-pollution clouds are shown to have enhanced overall inhomogeneity, with flight L2 being solely responsible for this enhanced inhomogeneity. Analysis suggests cloud age plays a larger role in the amount of inhomogeneity experienced than the aerosol number concentration, with dissipating clouds showing increased inhomogeneities as compared to growing or mature clouds. Results using a single, vertically developed cumulus cloud demonstrate enhanced droplet inhomogeneity near cloud top as compared to cloud base.
Highlights
The spatial inhomogeneity of cloud droplets at different spatial scales has impacts on multiple cloud processes, including precipitation formation on the smallest scales and radiative heating and cooling on the largest spatial scales
pair-correlation function (PCF) functions for L1, L2, H1, and H2 are given in Fig. 5, moving from Fig. 5a to d, respectively, with blue representing cloud edge data
Flight data obtained from the Center for Interdisciplinary Remotely Piloted Aircraft Studies (CIRPAS) Twin otter aircraft flown during the GoMACCS campaign near Houston, TX, from 2006 were used to investigate 81 non-precipitating cumulus clouds, and one vertically developed cumulus cloud, to better understand how droplet inhomogeneity changes as a function of cloud location and aerosol number concentration
Summary
The spatial inhomogeneity of cloud droplets at different spatial scales has impacts on multiple cloud processes, including precipitation formation on the smallest scales (millimeter to centimeter scale, from here on termed inertial clustering or just clustering) and radiative heating and cooling on the largest spatial scales. The work presented here deals with in situ measurements of the magnitude of cloud droplet spatial inhomogeneities at scales of centimeters to tens of meters (from here on termed droplet inhomogeneities or just inhomogeneities) to provide information on how the entrainment mixing present at cloud–clear air interfaces impacts inertial particles (i.e., cloud droplets). This information is of interest due to the complex physical processes controlling clouds, in particular the formation of precipitation and aerosol–cloud interactions, both of which can affect cloud lifetime and size. This is due to uniform condensational growth of cloud droplets leading to a narrowing of the drop size distri-
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