Abstract

Buoyancy-assisted droplet formation in a quiescent continuous phase is an effective technique to produce highly monodispersed droplets, especially millimetric droplets. A comprehensive study combining visualization experiment and numerical simulation was carried out to explore the underlying physics of single droplet generation in a buoyancy-assisted microfluidic device. Typical regimes, including dripping and jetting, were examined to gain a deep insight into the hydrodynamic difference between the regimes. Particularly, the transition from dripping regime to jetting regime was investigated to give an in-depth understanding of the transitional behaviors. The effects of interfacial tension coefficient on the droplet size and formation regimes are discussed, and a regime diagram is summarized. The results show that oscillation of the interface in dripping regimes after detachment is caused by the locally accelerated fluid during the neck pinching process. Droplet formation patterns with the characteristics of both dripping regime and jetting regime are observed and recognized as the transitional regime, and the interface oscillation lasts longer than that in dripping regime, implying intensive competition between interfacial tension and inertial force. Reducing interfacial tension coefficient results in the dripping-to-jetting transition occurring at a lower flow rate of the dispersed phase. The regime diagram indicates that only the inertial force is the indispensable condition of triggering the transition from dripping to jetting.

Highlights

  • Monodispersed emulsions are favorable in various applications, including inertial confinement fusion (ICF) target fabrication [1,2], cosmetics [3], drug delivery [4,5,6] and biological assays [7,8,9]

  • Interfacial tension, viscous force from the continuous phase and inertial force from the dispersed phase dominate the formation of droplets in the microfluidic devices [29]

  • Though numerous studies have been conducted exploring the performance of buoyancy-assisted microfluidic devices, most have been focused on experimental measurement and theoretical prediction based on force balancing

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Summary

Introduction

Monodispersed emulsions are favorable in various applications, including inertial confinement fusion (ICF) target fabrication [1,2], cosmetics [3], drug delivery [4,5,6] and biological assays [7,8,9]. Interfacial tension, viscous force from the continuous phase and inertial force from the dispersed phase dominate the formation of droplets in the microfluidic devices [29]. Due to the capability of producing monodispersed millimetric droplets, which is essential in applications that require big droplets, such as fabricating ICF targets [39], buoyancy-assisted droplet formation has once again attracted intensive attention. Though numerous studies have been conducted exploring the performance of buoyancy-assisted microfluidic devices, most have been focused on experimental measurement and theoretical prediction based on force balancing. The underlying mechanism of the transition behavior still lacks in-depth investigation, which is essential in formulating the control strategies during droplet formation In this context, combined efforts of visualization experiment and numerical simulation were conducted to clarify the transition from dripping regime to jetting regime in the buoyancy-assisted microfluidics. The effect of both Weber number and Bond number are discussed and summarized in a regime diagram

Experimental Setup
Mathematical Model
Numerical Solution
Dripping
Jetting
Dripping-to-Jetting Transition
Effect of Interfacial Tension Coefficient
Regime Diagram
Findings
Conclusions
Full Text
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