Abstract
The use of microwave double resonance for the analysis of difficult spectra is illustrated by the assignment of triazole through the identification of sequences of double-resonances. The rotational constants suggest that the assigned spectrum arises from 1,2,3-triazole, rather than the tautomeric form 1,2,5-triazole. The molecule has a planar equilibrium configuration and a dipole moment with its predominant component in the a-axis.Double resonance instrumentation is described in some detail and more general applications of the method are evaluated briefly.
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