Abstract
Simultaneous stimulated Raman scattering at the 992 cm−1 and the 3063 cm−1 line of benzene is observed by mode-locked ruby laser pulse excitation. The double line stimulated Raman scattering is initiated by self-focusing. The influence of small-scale self-focusing, self-phase modulation, and cross-phase modulation on the double line stimulated Raman scattering is discussed. At low pump pulse intensities, before the onset of small-scale self-focusing, the steady-state Raman gain factors of both Raman lines are determined by Raman energy conversion efficiency measurements.
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