Abstract
Measurements of temperature dependencies of the effective quadratic electrooptic coefficients n o 3 | g 1111 - g 2211 | and | n o 3 g 1111 - n e 3 g 3311 | in deuterated KDP are presented. The effective coefficients are found to decrease in a different way with temperature. This is explained in terms of different contributions of hydrogen bonds to the individual coefficients g 1111, g 2211, and g 3311. The results obtained indicate that for optical phenomena related to the third-order susceptibility descriptions based only on contributions of PO 4 tetrahedra are not precise enough.
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