Abstract

The perovskite oxide EuTiO3 (ETO) has attracted increased scientific interest due to its potential multiferroic properties and magnetic activity above and below its structural phase transition at TS=282 K. Various experiments have indirectly evidenced that this transition is neither a cubic tetragonal nor the only one occurring in ETO. Here, we show results demonstrating two further instabilities below TS based on lattice dynamics and spin-phonon interactions combined with a Landau free energy model with coupled order parameters. The transition temperatures agree with available experimental data where further instabilities have been anticipated. Published by the American Physical Society 2024

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