Abstract
The harmonic oscillator model is used in the derivation of general functions describing the distribution of molecules with excited vibrational levels formed as a result of chemical reactions. Allowance is made for the vibration-vibrational (v-v) exchange and vibration-translational (v-t) relaxation. Specific reactions are considered and it is shown that the formulas obtained can be used to calculate the population inversion density and unsaturated gain for any vibration-rotational transition of a laser-active molecule.
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