Abstract
The frequency dependence of the dissociation rate of the OsO 4 molecule by a strong infrared resonant field is shown to have a rich structure due to multiple photon absorption resonances. This permits laser isotope separation with small isotope shift. No dissociation was observed in the case of excitation of the R branch of the v 3 mode in OsO 4. Threshold characteristics of the dissociation have been studied as well.
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