Abstract

We theoretically investigate the effect of static disorder on the dynamics of photoexcited states in one-dimensional Mott insulators. We numerically calculate the time development of the state excited by a light pulse in the Pariser-Parr-Pople model, where disorder is introduced in the site energy and the transfer integral. In the weaker excitation case, the spin-charge coupling is induced by the disorder in the transfer integral. The effects of the disorder in the site energy on the spin-charge coupling are much weaker than those in the transfer integral. In the stronger excitation case, the spin and the charge degrees of freedom are coupled in the photoexcited states even in regular systems. The spin relaxations are enhanced by the disorders, and there are no significant differences in the effects of disorders on the spin relaxations between these two kinds of disorders.

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