Abstract

Natural catalysts used in the synthesis of carbon nanotubes have significant cost advantages due to their huge reserves, but natural minerals often require complicated pretreatments to obtain satisfactory products. In this study, red sandstone was directly used as a catalyst for the synthesis of multi-carbon nanotubes by chemical vapor deposition without complicated pretreatment. The SEM, TEM, Raman and TG characterization of the products at different growth temperatures ([Formula: see text]C, [Formula: see text]C and [Formula: see text]C) showed that [Formula: see text]C is the optimal condition for the growth of multi-walled carbon nanotubes (MWCNTs) by red sandstone. High-quality multi-wall carbon nanotubes can be obtained with a relatively high yield, and the [Formula: see text] of the product reaches 1.78, which exceeds that of many commercial multi-wall carbon nanotubes. Compared with other natural materials as catalysts for the synthesis of MWCNTs, red sandstone has a huge cost advantage because it can catalyze the synthesis of high-quality MWCNTs at [Formula: see text]C without complicated pretreatment.

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