Abstract
AbstractThe directional self‐assembly of exfoliated layered europium hydroxide (LEuH) nanosheets and europium‐containing heteropolytungstate anions has been achieved by mixing an LEuH colloidal solution and a Na9EuW10O36·32H2O (EuW10) solution at room temperature leading to the formation of a new inorganic/inorganic hybrid material, Eu2(OH)5(EuW10O36)0.11·5.5H2O (LEuH‐EuW10). The use of LEuH‐EuW10 in extractive catalytic oxidative desulfurization (ECODS) showed that highly efficient and selective deep desulfurization can be achieved in only 15 min under mild conditions. A maximum turnover number (TON) of around 1600 has been achieved. In addition, the catalyst can be recycled and reused at least 10 times with only a slight loss of catalytic efficiency.
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