Abstract
The direct non-oxidative methane aromatization over commercially available gallium nitride powder has been investigated for the first time in a fixed bed reactor under continuous operation. Gallium nitride catalyst is highly active. High reaction temperatures (650–710°C) are needed to initiate benzene formation due to the small surface area (8m2g−1) of the gallium nitride material, thermodynamic constraints and the low residence time (1–4s). Besides benzene and toluene, C2 species and coke were formed.
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