Abstract
The vibrational predissociation lifetime of NeBr 2 in the ground electronic state with one vibrational quantum in the halogen stretch was measured directly in a free jet expansion. NeBr 2(X, ν = 1) was detected by optical-optical double resonance to monitor the population as a function of distance from the nozzle to the laser interaction region. The vibrational predissociation lifetime for NeBr 2(X, ν = 1) was determined to be 8 ± 3 μs.
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