Abstract

Using the technique of neutron spin-echo spectroscopy, we have conducted a direct measurement of the superparamagnetic relaxation of nanoscale, magnetic monodomain iron particles in the time range between 0.01 and 160 nsec and for momentum transfers $q$ between 0.035 and $0.15{\AA{}}^{\ensuremath{-}1}$. Using a phenomenological model which includes the effect of a particle size distribution, we are able to determine the temperature $T$ and $q$ dependence of the longitudinal superspin relaxation time spanning 4 orders of magnitude. We find that for $T\ensuremath{\lesssim}40\mathrm{K}$, interparticle correlations affect the longitudinal superspin fluctuations.

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